I don't think leaving your current role before securing something new would be a wise idea. It would likely be more damaging for your mental health as you'd feel a lack of purpose, not have a routine, and may find yourself unemployed for a while which could end up impacting your confidence and self-esteem.
I saw another one of your post where you'd expressed interest in becoming a Paramedic, and your reasons for why that may not be possible. How about training to be a Nurse instead? There are so many different specialisms that you could choose, and it offers plenty of opportunities in the UK and globally. If you specialised as an ER Nurse you would have some similarities to being a Paramedic because of the pace, variety, working with multidisciplinary colleagues, and it being emergency medicine.